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• W3087524492 startingPage "1535" @default.
• W3087524492 abstract "Spirocyclic Ag9 clusters, as a new form of intrinsically chiral metal clusters, were constructed through vertex-sharing of two in-situ-generated heteroaryl diide-centered metal rings. Such core-peripheral type clusters exhibit versatile photoluminescent and chiroptical behavior under different aggregation conditions. In contrast to a ligand-based fluorescence emission in a diluted solution of the clusters, a solvent polarity-caused assembly gives rise to new cluster-based phosphorous luminescence owing to radiative mode switching and aggregation-induced emission. Assembly of cluster enantiomers leads to micrometer-long helical nanofibers, whose handedness is determined by absolute configuration of individual spirocyclic clusters. Benefiting from exciton couplings of helical arrangements of chelating ligands at molecular and microscopic levels, the assembled film of cluster enantiomers exhibits circularly polarized luminescence with a high anisotropy factor (0.16)." @default.
• W3087524492 created "2020-09-25" @default.
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• W3087524492 date "2020-11-16" @default.
• W3087524492 modified "2023-10-11" @default.
• W3087524492 title "Assembly‐Induced Strong Circularly Polarized Luminescence of Spirocyclic Chiral Silver(I) Clusters" @default.
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• W3087524492 doi "https://doi.org/10.1002/anie.202008765" @default.
• W3087524492 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/32959488" @default.
• W3087524492 hasPublicationYear "2020" @default.
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