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- W3087759782 endingPage "106592" @default.
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- W3087759782 abstract "The high yields of coke and tar pitch relating to volatile reactions can cause plug in the product lines during low temperature pyrolysis of low-rank coals. To study the potential transformation of volatile into coke during its migration in the pyrolysis process, six distillates and their blends from the same coal tar were heated at 400–600 °C. The composition, radicals of six distillates and coke structure were characterized by GC × GC–MS, ESR and Raman techniques, respectively. The results show that the coke yields increase with temperature during thermal reaction for all six distillates. When light oil and pitch are blended, the interaction between the two distillates compresses the transformation of volatile into coke above 500 °C. This can be ascribed to that the reactive hydrogen radicals generated from light oil may weaken the bonding between large molecules. By contrast, other distillates (phenolic oil, naphthalic oil, wash oil and anthracene oil) promote coke formation, resulting in higher coke yields than expected. It is also observed that the highest extent of interaction occurs between phenolic oil and pitch, which may be related to the high content of oxygen containing compounds in phenolic oil and the high electron density of the compounds in pitch. • Coke yield of all six distillates from coal tar increases with temperature. • Interaction of pitch with light oil compresses coke yield above 500 °C. • Interaction of pitch with distillates except for light oil increases coke yield. • The blend of pitch and phenolic oil shows the highest interaction for forming coke." @default.
- W3087759782 created "2020-09-25" @default.
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- W3087759782 date "2021-01-01" @default.
- W3087759782 modified "2023-09-24" @default.
- W3087759782 title "Insights into coke formation during thermal reaction of six different distillates from the same coal tar" @default.
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- W3087759782 doi "https://doi.org/10.1016/j.fuproc.2020.106592" @default.
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