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- W3087888032 abstract "Substrate-supported metal–organic frameworks (MOFs) films are desired to realize their potential in practical applications. Herein, a novel substrate-seeding secondary-growth strategy is developed to prepare composites of uniform MOFs films on aerogel walls. Briefly, the organic ligand is “pre-seeded” onto the aerogel walls, and then a small amount of metal-ion solution is sprayed onto the prepared aerogel. The sprayed solution diffuses along the aerogel walls to form a continuous thin layer, which confines the nucleation reaction, promoting the formation of uniform MOFs films on the aerogel walls. The whole process is simple in operation, highly efficient, and eco-friendly. The resulting hierarchical MOFs/aerogel composites have abundant accessible active sites and enable excellent mass transfer, which endows the composite with outstanding catalytic activity and stability in both liquid-phase CO2 cycloaddition and electrochemical oxygen evolution reaction (OER) process." @default.
- W3087888032 created "2020-10-01" @default.
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- W3087888032 date "2020-11-09" @default.
- W3087888032 modified "2023-10-03" @default.
- W3087888032 title "Preparation of MOF Film/Aerogel Composite Catalysts via Substrate‐Seeding Secondary‐Growth for the Oxygen Evolution Reaction and CO <sub>2</sub> Cycloaddition" @default.
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- W3087888032 doi "https://doi.org/10.1002/anie.202012354" @default.
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