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- W3087906280 abstract "Dielectric permittivity is central to many biological and physiochemical systems, as it affects the long-range electrostatic interactions. Similar to many fluid properties, confinement greatly alters the dielectric response of polar liquids. Many studies have focused on the reduction of the dielectric response of water under confinement. Here, using molecular dynamics simulations, statistical-mechanical theories, and multiscale methods, we study the out-of-plane (z-axis) dielectric response of protic and aprotic fluids confined inside slit-like graphene channels. We show that the reduction in perpendicular permittivity is universal for all the fluids and exhibits a Langevin-like behavior as a function of channel width. We show that this reduction is due to the favorable in-plane (x-y plane) dipole-dipole electrostatic interactions of the interfacial fluid layer. Furthermore, we observe an anomalously low dielectric response under an extreme confinement." @default.
- W3087906280 created "2020-10-01" @default.
- W3087906280 creator A5029571026 @default.
- W3087906280 creator A5073593948 @default.
- W3087906280 date "2020-09-23" @default.
- W3087906280 modified "2023-10-14" @default.
- W3087906280 title "Universal Reduction in Dielectric Response of Confined Fluids" @default.
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- W3087906280 doi "https://doi.org/10.1021/acsnano.0c03173" @default.
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- W3087906280 hasPublicationYear "2020" @default.
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