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- W3088394015 abstract "A 36-nuclear Zr(IV) cluster based on six [Zr6O4(OH)4] units is found to form three different crystal structures depending on synthesis conditions. The cubic phase (ZF-3c) is obtained when the cyclic clusters are interlinked by Na+ or K+ ions. In the absence of alkali metal ions, either tetragonal (ZF-3t) or hexagonal (ZF-3h) packing structures are formed. All the solids remain crystalline after evacuation, and ZF-3h possesses a permanent porosity. Upon repeated adsorptions of water vapor, the three different molecular solids comprising the same building blocks turn amorphous; however, overall uptake properties are not deteriorated and reproducible isotherms are observed featuring fast uptake at low relative humidity and unrestricted uptake at RH > 90%. A good reproducibility has also been established in cyclic adsorption–desorption measured under dynamic flow conditions, and, especially ZF-3t displays the working capacity 2.7 times that of zeolite 4A thanks to the fast desorption kinetics." @default.
- W3088394015 created "2020-10-01" @default.
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- W3088394015 date "2020-09-20" @default.
- W3088394015 modified "2023-10-18" @default.
- W3088394015 title "Static and Dynamic Adsorptions of Water Vapor by Cyclic [Zr <sub>36</sub> ] Clusters: Implications for Atmospheric Water Capture Using Molecular Solids" @default.
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- W3088394015 doi "https://doi.org/10.1002/bkcs.12100" @default.
- W3088394015 hasPublicationYear "2020" @default.
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