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- W3089015372 endingPage "110432" @default.
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- W3089015372 abstract "The construction of heterostructure composites is an efficient way to widen the spectral response range and reduce the photogenerated electrons-holes recombination, but it is still a challenge to realize the maximizing the photocatalytic performance of different photoresponsive material, especially at low temperature. In this work, we construct a series of [email protected]/MA composites by first designing a series of [email protected]@MA sandwich templates and then calcining these sandwich templates at high temperature. During the pyrolysis process, ZIF-8 and melamine precursors would convert into ZnO and gCN structure so as to form the [email protected] composite at high temperature, while urea molecular would decompose to release ammonia molecules which rush out from the interior of ZIF-8 to make the [email protected]/MA composites become fluffy and porous. Detailed characterization results reveal that the [email protected]/MA composites exhibit enhanced spectral response range and the lower charge-carrier recombination rates. When being used in photocatalytic oxidative coupling of amines at low temperature under air condition, the optimal ZnO(0.1)@gCN-UA/MA catalyst exhibits excellent activity, affording the imine product with 96% yield. Moreover, the catalysts also exhibit a wide substrate compatibility and recyclability." @default.
- W3089015372 created "2020-10-01" @default.
- W3089015372 creator A5034458835 @default.
- W3089015372 creator A5065765224 @default.
- W3089015372 date "2020-11-01" @default.
- W3089015372 modified "2023-09-26" @default.
- W3089015372 title "Sandwich template derived porous ZnO@gCN heterostructure nanocomposites and the enhanced photocatalytic efficiency in oxidative coupling of amines" @default.
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- W3089015372 doi "https://doi.org/10.1016/j.optmat.2020.110432" @default.
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