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- W3089478255 abstract "We report herein the diversity-oriented synthesis of various tetracyclic Isodon diterpenoid scaffolds guided by radical cyclization logic. Our substrate-based dienyne radical cyclization approach is distinctive from reagent-based rearrangement approaches that are generally applied in biosynthesis or previous synthetic studies. An unprecedented cyclization at C14 via 1,5-radical translocation/5-exo-trig cyclization is observed, which enriches our radical cyclization pattern. Furthermore, biological evaluations revealed that several new natural product-like compounds showed promising anticancer activities against various cancer cell lines." @default.
- W3089478255 created "2020-10-08" @default.
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- W3089478255 date "2020-10-06" @default.
- W3089478255 modified "2023-10-16" @default.
- W3089478255 title "Syntheses of Skeletally Diverse Tetracyclic <i>Isodon</i> Diterpenoid Scaffolds Guided by Dienyne Radical Cyclization Logic" @default.
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- W3089478255 doi "https://doi.org/10.1021/acs.orglett.0c02920" @default.
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