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• W3089545810 abstract "Hybrid organic–inorganic perovskites (HOIPs) with chiral organic ligands exhibit highly spin-dependent transport and strong natural optical activity (NOA). Here we show that these remarkable features can be traced to a chirality-induced spin–orbit coupling (SOC), Hso = ατkzσz, which connects the carrier’s spin (σz), its wave vector (kz), and the material’s helicity (τ) along the screw direction with strength α controlled by the geometry of the organic ligands. This SOC leads to a macroscopic spin polarization in the presence of an electrical current and is responsible for the observed spin-selective transport. NOA originates from a coupling between the exciton’s center-of-mass wave vector Kz and its circular polarization jzex, Hso′ = α′τKzjzex, contributed jointly from the electron’s and the hole’s SOCs in an exciton. Our model provides a roadmap to achieve a strong and tunable chirality in HOIPs for novel applications utilizing carrier spin and photon polarization." @default.
• W3089545810 created "2020-10-08" @default.
• W3089545810 creator A5017944235 @default.
• W3089545810 date "2020-09-29" @default.
• W3089545810 modified "2023-10-16" @default.
• W3089545810 title "Chirality-Induced Spin–Orbit Coupling, Spin Transport, and Natural Optical Activity in Hybrid Organic–Inorganic Perovskites" @default.
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• W3089545810 doi "https://doi.org/10.1021/acs.jpclett.0c02589" @default.
• W3089545810 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/32991181" @default.
• W3089545810 hasPublicationYear "2020" @default.
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