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• W3089808329 endingPage "4400" @default.
• W3089808329 startingPage "4391" @default.
• W3089808329 abstract "The 2,5‐, 2,6‐, and 3,5‐pyridinedicarboxylic (2,5‐, 2,6‐ and 3,5‐pydcH 2 ), and 2,3‐pyrazinedicarboxylic (2,3‐pyzdcH 2 ) acids have been used to synthesize six uranyl ion complexes including various counterions under solvo‐hydrothermal conditions. While [NH 4 ] 2 [UO 2 (2,6‐pydc) 2 ] · 3H 2 O ( 1 ) is a discrete, mononuclear species, [UO 2 (2,6‐pydc) 2 Cu( R,S ‐Me 6 cyclam)] ( 2 ) crystallizes as a monoperiodic coordination polymer through axial bonding of copper(II) to carboxylate donors. [PPh 3 Me][UO 2 (OH)(2,5‐pydc)] · H 2 O ( 3 ) and [Ni( R,S ‐Me 6 cyclam)][UO 2 (OH)(2,5‐pydc)] 2 · 2H 2 O ( 4 ) contain di‐hydroxo‐bridged dinuclear uranyl subunits assembled into homometallic, monoperiodic polymers. [(UO 2 ) 2 (3,5‐pydc) 2 (HCOO) 2 Ni( R,S ‐Me 6 cyclam)] ( 5 ) crystallizes as a heterometallic diperiodic network with the V 2 O 5 topology, and [PPh 4 ][UO 2 (OH)(2,3‐pyzdc)] ( 6 ) is a diperiodic species with sql topology. All complexes have well‐resolved uranyl emission spectra in the solid state, and three of them have photoluminescence quantum yields among the highest reported for uranyl carboxylate complexes, 44 % for 1 , 71 % for 3 , and 36 % for 6 ." @default.
• W3089808329 created "2020-10-08" @default.
• W3089808329 creator A5018099405 @default.
• W3089808329 creator A5026641338 @default.
• W3089808329 creator A5039862779 @default.
• W3089808329 creator A5049479234 @default.
• W3089808329 creator A5063941923 @default.
• W3089808329 creator A5073854687 @default.
• W3089808329 date "2020-10-28" @default.
• W3089808329 modified "2023-09-25" @default.
• W3089808329 title "Optimizing Photoluminescence Quantum Yields in Uranyl Dicarboxylate Complexes: Further Investigations of 2,5‐, 2,6‐ and 3,5‐Pyridinedicarboxylates and 2,3‐Pyrazinedicarboxylate" @default.
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