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- W3090293860 abstract "Abstract This chapter reviews the fundamentals and recent progress in the understanding of the molecular electrical doping of organic semiconductors; that is, the doping of conjugated polymers (CPs) and conjugated molecules (COMs). In contrast to inorganic semiconductors, the potential of using doping to improve the performance of organic electronic devices has been established only in the last decade, however, with resounding success. Doping COMs and CPs allows both increasing conductivity by orders of magnitude and tuning their energy levels to reduce energy barriers for charge transport. In this chapter, we focus on the broad range of phenomena observed upon doping organic semiconductors and highlight two distinctly different scenarios: the immediate, pairwise formation of ions and the formation of ground-state charge transfer complexes between the semiconductor and the dopant through supramolecular hybridization of their respective frontier molecular orbitals. Doping-related modifications of the organic semiconductor density of states and conditions for carrier release after the initial charge transfer are discussed, spectroscopic evidence for the underlying processes at work are summarized and correlations between the respective doping scenario and the underlying microstructure are highlighted. This chapter is a carefully revised and updated version of Hase, H., Salzmann, I., 2019. Doping in organic semiconductors. In: Ostroverkhova, O. (Ed.), Handbook of organic materials for electronic and photonic devices, second ed., Woodhead Publishing, pp. 349–383, https://doi.org/10.1016/B978-0-08-102284-9.00011-5 ." @default.
- W3090293860 created "2020-10-08" @default.
- W3090293860 creator A5058614286 @default.
- W3090293860 creator A5060252474 @default.
- W3090293860 creator A5071257801 @default.
- W3090293860 date "2021-01-01" @default.
- W3090293860 modified "2023-09-27" @default.
- W3090293860 title "Chemical doping of organic semiconductors" @default.
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