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• W3090765668 abstract "Tracer diffusion coefficients D* of lithium ions in LixMn2O4 (0.2 < x < 1) thin films were measured as a function of the composition x by using secondary ion mass spectrometry. For this purpose, a new “step-isotope-exchange method” was developed to observe the time dependence of the 6Li isotope concentration ratio in the LixMn2O4 film which is in contact with a 6Li-enriched electrolyte to exchange Li+ ions. A steep decrease in D* depending on the Li composition was observed for LixMn2O4, with D* = 8 × 10–13 cm2 s–1 for x = 0.2 and decreasing to 1.5 × 10–17 cm2 s–1 for x = 1.0 (bulk diffusion coefficient, Db*). This behavior is well explained by a vacancy diffusion model for the α phase on LixMn2O4 (0.77 < x < 1.0). Chemical diffusion coefficients D̃ were also measured in the range of 0.2 < x < 1.0 by an electrochemical method, which was compared with the D* to evaluate the effect of thermodynamic factors. The thermodynamic factors and interactions between Li+ ions were found to strongly influence the chemical diffusion coefficient. The tracer diffusion measurements are important to understand the charge–discharge mechanism in the electrodes of lithium-ion batteries." @default.
• W3090765668 created "2020-10-08" @default.
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• W3090765668 date "2020-09-29" @default.
• W3090765668 modified "2023-10-17" @default.
• W3090765668 title "Tracer Diffusion Coefficients of Li Ions in Li_<i>x</i>Mn₂O₄ Thin Films Observed by Isotope Exchange Secondary Ion Mass Spectrometry" @default.
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• W3090765668 doi "https://doi.org/10.1021/acs.jpcc.0c06375" @default.
• W3090765668 hasPublicationYear "2020" @default.
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