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- W3090905609 abstract "Molecular structure of an organic photocatalist, 9-mesityl-10-methylacrinium cation, at a photo-induced electron-transferred state was directly observed by a pump-probe single crystal X-ray structure analysis. Observed photo-induced structural changes were the bending of the N-methly group and the positional change of perchrolate anion, which co-exists in the crystal. Those structural changes respectively represented the reduction of the 10-methylacridinium cation and the oxidation of the mesitylene by photo-induced electron transfer. The dyhedral angle betweem 10-methylacridinium and mesitylene moieties at the electron-transferred state was almost identical with the ground one. This is a clear evidence for restriction of intramolecular back electron transfer and long-lived character of the electron-transferred state. The observed geometrical features will provide a solid basis for designing a novel artificital photosynthetic system." @default.
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- W3090905609 date "2013-01-01" @default.
- W3090905609 modified "2023-09-26" @default.
- W3090905609 title "Visualization of an Organic Photocatalyst ‘in Action’ by a Pump-Probe Single Crystal X-ray Structure Analysis" @default.
- W3090905609 doi "https://doi.org/10.5940/jcrsj.55.2" @default.
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