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- W3091539554 abstract "Developing highly-effective catalysts through a facile method for activating peroxymonosulfate (PMS) to degrade recalcitrant pollutants is highly desirable. In this work, porous carbon-coated iron-manganese oxides ([email protected]) was facilely synthesized. The porous carbon film on the surface of [email protected] was beneficial to adsorption of bisphenol A (BPA) and flow of electrons. The catalytic degradation performance toward BPA was significantly improved with the increase of surface roughness and porosity of [email protected] after calcination. In particular, [email protected] derived at 300 °C ([email protected]) exhibited the highest degradation rate benefiting from the existence of Mn2O3. More than 95% BPA could be removed in 30 min by [email protected]/PMS system and remained efficient in a wide pH range from 3.0 to 10.0, especially in alkaline conditions. The intermediates of BPA degradation were identified and the degradation pathways involved hydroxyl oxidation and benzene ring-opening were proposed based on GC–MS results. The removal rate of BPA can maintain more than 80% following five cycles. Thus, the as-prepared [email protected] composites are available to serve as efficient and eco-friendly catalysts for advanced catalytic oxidation of recalcitrant pollutants." @default.
- W3091539554 created "2020-10-08" @default.
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- W3091539554 date "2021-02-01" @default.
- W3091539554 modified "2023-10-15" @default.
- W3091539554 title "Surface-active MnFeO@C cubes as enhanced peroxymonosulfate activators for efficient degradation of bisphenol A" @default.
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- W3091539554 doi "https://doi.org/10.1016/j.apsusc.2020.148008" @default.
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