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• W3092048634 abstract "Electrochemical N₂ reduction is an environmentally friendly and sustainable approach for NH₃ synthesis under mild conditions, while an efficient electrocatalyst is crucial for the N₂ reduction reaction (NRR). Herein, we report Ti³⁺ self-doped TiO₂₋ₓ nanowires on Ti mesh (Ti³⁺–TiO₂₋ₓ/TM) as an efficient non-noble-metal NRR electrocatalyst with excellent selectivity. In 0.1 M Na₂SO₄, the Ti³⁺–TiO₂₋ₓ/TM achieves a high faradaic efficiency of 14.62% with a NH₃ yield of 3.51 × 10⁻¹¹ mol s⁻¹ cm⁻² at −0.55 V vs. the reversible hydrogen electrode. Density functional theory calculations further reveal that introducing Ti³⁺ decreases the reaction energy barrier and increases the number of active sites on the TiO₂ surface for the NRR." @default.
• W3092048634 created "2020-10-15" @default.
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• W3092048634 date "2020-01-01" @default.
• W3092048634 modified "2023-10-05" @default.
• W3092048634 title "Ti³⁺ self-doped TiO₂₋ₓ nanowires for efficient electrocatalytic N₂ reduction to NH₃" @default.
• W3092048634 hasPublicationYear "2020" @default.
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