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• W3092750322 startingPage "2964" @default.
• W3092750322 abstract "We report an artificial molecular machine that moves along a track, iteratively joining building blocks to form an oligomer of single sequence with a continuous backbone of carbon-carbon bonds. The rotaxane features a macrocycle bearing an aldehyde-terminated chain and an axle containing different phosphonium ylides separated by rigid spacers. Each ylide is large enough to block the passage of the macrocycle, trapping the ring between the stopper at the terminus of original threading and the next ylide along the track. Once a building block is reachable, it is removed from the track through a Wittig reaction that adds it to the terminus of the growing chain. Operation on a four-barrier tetra(phosphonium salt) track produces a tetra(diphenylpropane) of single sequence linked through alkene bonds. The prototype extends the principle for molecular machines that build polymers by moving along tracks to the synthesis of sequence-encoded chains with continuous carbon backbones." @default.
• W3092750322 created "2020-10-22" @default.
• W3092750322 creator A5014852936 @default.
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• W3092750322 creator A5074088076 @default.
• W3092750322 date "2020-11-01" @default.
• W3092750322 modified "2023-10-18" @default.
• W3092750322 title "A Track-Based Molecular Synthesizer that Builds a Single-Sequence Oligomer through Iterative Carbon-Carbon Bond Formation" @default.
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• W3092750322 doi "https://doi.org/10.1016/j.chempr.2020.09.021" @default.
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