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- W3092972015 abstract "Abstract Electrolytic water splitting to generate hydrogen and oxygen is one of the most promising ways in which to harness intermittent renewable power sources and store the energy these provide as a clean‐burning and sustainable fuel. In recent years, this has led to an explosion in reports on electrochemical water splitting, most of them focused on improving the efficiency of the electrochemical reactions themselves. However, efficient generation of hydrogen and oxygen is of little use if these products cannot be kept separate and the community is now coming to realize that there are considerable challenges associated with maintaining adequate separation between H 2 and O 2 during electrolysis driven by intermittent renewable sources. Decoupled electrolysis (whereby oxygen production occurs with reduction of a suitable mediator and hydrogen production is then paired with the reoxidation of this mediator) offers a solution to many of these challenges by allowing O 2 and H 2 to be produced at different times, at different rates, and even in completely different electrochemical cells. In this review, an overview of recent progress in the field of decoupled electrolysis for water splitting is given and the potential that this approach has for enabling a range of other sustainable chemical processes is explored." @default.
- W3092972015 created "2020-10-22" @default.
- W3092972015 creator A5002833191 @default.
- W3092972015 creator A5024797516 @default.
- W3092972015 creator A5055879607 @default.
- W3092972015 date "2020-10-13" @default.
- W3092972015 modified "2023-10-16" @default.
- W3092972015 title "Decoupled Electrochemical Water Splitting: From Fundamentals to Applications" @default.
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- W3092972015 doi "https://doi.org/10.1002/aenm.202002453" @default.