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• W3093472231 abstract "We prove complete controllability for rotational states of an asymmetric top molecule belonging to degenerate values of the orientational quantum number M. Based on this insight, we construct a pulse sequence that energetically separates population initially distributed over degenerate M-states, as a precursor for orientational purification. Introducing the concept of enantio-selective controllability, we determine the conditions for complete enantiomer-specific population transfer in chiral molecules and construct pulse sequences realizing this transfer for population initially distributed over degenerate M-states. This degeneracy presently limits enantiomer-selectivity for any initial state except the rotational ground state. Our work thus shows how to overcome an important obstacle towards separating, with electric fields only, left-handed from right-handed molecules in a racemic mixture." @default.
• W3093472231 created "2020-10-22" @default.
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• W3093472231 date "2020-10-19" @default.
• W3093472231 modified "2023-09-27" @default.
• W3093472231 title "Complete Controllability Despite Degeneracy: Quantum Control of Enantiomer-Specific State Transfer in Chiral Molecules" @default.
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• W3093472231 hasPublicationYear "2020" @default.
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