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- W3094159717 abstract "The dynamics of materials slow as the temperature is cooled to the glass transition temperature ( T g ). The rapidity at which the equilibrium dynamics slow upon cooling is known as fragility, if evaluated at T g . The measurement of fragility in various glassy systems is a huge body of research, with discrepancies in measured fragility values being common. This report reviews the mathematics behind determining fragility as it relates to glassy dynamics in polymers, small molecules, and inorganics. Various derivative plots are proposed that demonstrate how the fragility of a system is strongly dependent on chosen empirical constants such as T g . This includes visualizations of how fragility changes with the value chosen for T g or with the time constant τ g used to define T g , with τ g = 100 s being a common choice. Using poly(vinyl acetate) as an example, it is demonstrated how various factors affect the measurement of fragility." @default.
- W3094159717 created "2020-10-29" @default.
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- W3094159717 date "2021-02-01" @default.
- W3094159717 modified "2023-10-17" @default.
- W3094159717 title "Using derivative plots to ascertain fragilities of glass-formers" @default.
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- W3094159717 doi "https://doi.org/10.1016/j.jnoncrysol.2020.120478" @default.
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