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• W3094334662 abstract "Biohybrid photoelectrochemical systems could combine the light-harvesting ability of semiconductor photocatalysts and the CO2-processing capability of biocatalysts to realize CO2 reduction. How to develop the energy-utilized model can be of importance for the mechanism exploration of photosynthesis. Here, a biohybrid photoelectrochemical system based on HCOO--CO2 circulation was developed to realize the conversion both of solar-to-electric energy and chemical-to-electric energy. The device consists of a TiO2 nanoparticle photoanode and a laser-scribed graphene/formate dehydrogenase biocathode, which was utilized for the formic acid oxidation and the biocatalysis reduction of CO2 to HCOO-, respectively. The as-proposed biohybrid photoelectrochemical system exhibits good performance with an open-circuit potential of 0.93 V and a maximum power output density of 76 μW cm-2. This ingenious strategy not only exploits a robust carbon circulation system for the conversion of solar energy but also provides a way of constructing complex artificial photosynthesis systems." @default.
• W3094334662 created "2020-10-29" @default.
• W3094334662 creator A5015918308 @default.
• W3094334662 creator A5023277532 @default.
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• W3094334662 date "2020-10-22" @default.
• W3094334662 modified "2023-10-14" @default.
• W3094334662 title "Biohybrid Cells for Photoelectrochemical Conversion Based on the HCOO^––CO₂ Circulation Approach" @default.
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• W3094334662 doi "https://doi.org/10.1021/acsabm.0c01166" @default.
• W3094334662 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35019546" @default.
• W3094334662 hasPublicationYear "2020" @default.
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