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- W3094551844 abstract "To elevate the performance of polymer solar cells (PSC) processed by non-halogenated solvents, a dissymmetric fused-ring acceptor BTIC-2Cl-γCF3 with chlorine and trifluoromethyl end groups has been designed and synthesized. X-ray crystallographic data suggests that BTIC-2Cl-γCF3 has a 3D network packing structure as a result of H- and J-aggregations between adjacent molecules, which will strengthen its charge transport as an acceptor material. When PBDB-TF was used as a donor, the toluene-processed binary device realized a high power conversion efficiency (PCE) of 16.31 %, which improved to 17.12 % when PC71ThBM was added as the third component. Its efficiency of over 17 % is currently the highest among polymer solar cells processed by non-halogenated solvents. Compared to its symmetric counterparts BTIC-4Cl and BTIC-CF3-γ, the dissymmetric BTIC-2Cl-γCF3 integrates their merits, and has optimized the molecular aggregations with excellent storage and photo-stability, and also extending the maximum absorption peak in film to 852 nm. The devices exhibit good transparency indicating a potential utilization in semi-transparent building integrated photovoltaics (ST-BIPV)." @default.
- W3094551844 created "2020-10-29" @default.
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- W3094551844 date "2020-12-10" @default.
- W3094551844 modified "2023-10-18" @default.
- W3094551844 title "17.1 %‐Efficient Eco‐Compatible Organic Solar Cells from a Dissymmetric 3D Network Acceptor" @default.
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- W3094551844 doi "https://doi.org/10.1002/anie.202013053" @default.
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