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• W3094683215 abstract "Recent developments in the synthesis of graphene-based structures focus on continuous improvement of porous nanostructures, doping of thin films, and mechanisms for the construction of three-dimensional architectures. Herein, we synthesize creeper-like Ni3Si2/NiOOH/graphene nanostructures via low-pressure all-solid melting-reconstruction chemical vapor deposition. In a carbon-rich atmosphere, high-energy atoms bombard the Ni and Si surface, and reduce the free energy in the thermodynamic equilibrium of solid Ni-Si particles, considerably catalyzing the growth of Ni-Si nanocrystals. By controlling the carbon source content, a Ni3Si2 single crystal with high crystallinity and good homogeneity is stably synthesized. Electrochemical measurements indicate that the nanostructures exhibit an ultrahigh specific capacity of 835.3 C g-1 (1193.28 F g-1) at 1 A g-1; when integrated as an all-solid-state supercapacitor, it provides a remarkable energy density as high as 25.9 Wh kg-1 at 750 W kg-1, which can be attributed to the free-standing Ni3Si2/graphene skeleton providing a large specific area and NiOOH inhibits insulation on the electrode surface in an alkaline solution, thereby accelerating the electron exchange rate. The growth of the high-performance composite nanostructure is simple and controllable, enabling the large-scale production and application of microenergy storage devices." @default.
• W3094683215 created "2020-11-09" @default.
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• W3094683215 date "2020-10-27" @default.
• W3094683215 modified "2023-10-16" @default.
• W3094683215 title "Superior Pseudocapacitive Storage of a Novel Ni3Si2/NiOOH/Graphene Nanostructure for an All-Solid-State Supercapacitor" @default.
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• W3094683215 doi "https://doi.org/10.1007/s40820-020-00527-w" @default.
• W3094683215 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/8187555" @default.
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• W3094683215 hasPublicationYear "2020" @default.
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