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- W3094947625 abstract "Abstract We resolve the real-time coherent rotational motion of isolated water molecules encapsulated in fullerene-C 60 cages by time-domain terahertz (THz) spectroscopy. We employ single-cycle THz pulses to excite the low-frequency rotational motion of water and measure the subsequent coherent emission of electromagnetic waves by water molecules. At temperatures below ~ 100 K, C 60 lattice vibrational damping is mitigated and the quantum dynamics of confined water are resolved with a markedly long rotational coherence, extended beyond 10 ps. The observed rotational transitions agree well with low-frequency rotational dynamics of single water molecules in the gas phase. However, some additional spectral features with their major contribution at ~2.26 THz are also observed which may indicate interaction between water rotation and the C 60 lattice phonons. We also resolve the real-time change of the emission pattern of water after a sudden cooling to 4 K, signifying the conversion of ortho-water to para-water over the course of 10s hours. The observed long coherent rotational dynamics of isolated water molecules confined in C 60 makes this system an attractive candidate for future quantum technology." @default.
- W3094947625 created "2020-11-09" @default.
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- W3094947625 date "2020-10-27" @default.
- W3094947625 modified "2023-10-05" @default.
- W3094947625 title "Rotational coherence of encapsulated ortho and para water in fullerene-C60 revealed by time-domain terahertz spectroscopy" @default.
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- W3094947625 doi "https://doi.org/10.1038/s41598-020-74972-3" @default.
- W3094947625 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/7592058" @default.
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