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- W3095784853 abstract "Hybrid catalysis, which combines chemo- and biocatalytic benefits, is an efficient way to address green chemistry principles. 5-Hydroxymethylfurfural (HMF) is a versatile building block in numerous industrial applications. To date, few studies have described the production of its amine derivatives and their polymers. Finding a good methodology to directly transform HMF to 5-aminomethyl-2-furancarboxylic acid (AMFC) therefore represents an important challenge. After selecting the best oxidation catalyst for HMF conversion to 5-aldehyde-2-furancarboxylic acid and immobilizing a transaminase onto a solid carrier, we implemented the first one-pot/two-steps hybrid catalytic process to produce AMFC (77 % yield); this is the most efficient AMFC catalytic production method from HMF reported to date. This process also produced 2,5-furandicarboxylic acid (21 % yield) as a major secondary product that can be applied to polymer syntheses such as polyethylene furanoate. Herein, we report a novel way to access new biosourced polymers based on HMF oxidized and aminated derivatives." @default.
- W3095784853 created "2020-11-09" @default.
- W3095784853 creator A5000172209 @default.
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- W3095784853 creator A5090093607 @default.
- W3095784853 date "2020-11-26" @default.
- W3095784853 modified "2023-09-24" @default.
- W3095784853 title "Hybrid Conversion of <i>5</i> ‐Hydroxymethylfurfural to <i>5</i> ‐Aminomethyl‐ <i>2</i> ‐furancarboxylic acid: Toward New Bio‐sourced Polymers" @default.
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- W3095784853 doi "https://doi.org/10.1002/cctc.202001446" @default.
- W3095784853 hasPublicationYear "2020" @default.