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• W3096483243 abstract "Original endocyclic enamides based on a bicyclic aza‐diketopiperazine (aza‐DKP) structure have been used as dienophile partners in the Povarov reaction. The reported method represents a successful strategy for the structural diversification of the aza‐DKP scaffold, giving access to a new family of fused tetracyclic N ‐heterocycles, which contain at least four nitrogen atoms in the heterocyclic structure. Depending on the nature of the aldehyde partner, the cycloadditions have been performed either as a two‐component or a three‐component Povarov reaction (2CPR or 3CPR), in the presence of BF 3 as a Lewis acid catalyst. With aliphatic aldehydes the reaction proceeds with high diastereoselectivities in favor of the cis compounds. Some mechanistic aspects of this cycloaddition have been examined computationally." @default.
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• W3096483243 date "2020-11-13" @default.
• W3096483243 modified "2023-10-10" @default.
• W3096483243 title "Endocyclic Enamides Derived from Aza‐Diketopiperazines as Olefin Partners in Povarov Reaction: An Access to Tetracyclic N‐Heterocycles" @default.
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• W3096483243 doi "https://doi.org/10.1002/ejoc.202001339" @default.
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