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• W3097349416 abstract "We report the first simulations of nonsolvent-induced phase separation (NIPS) that predict membrane microstructures with graded asymmetric pore size distribution. In NIPS, a polymer solution film is immersed in a nonsolvent bath, enriching the film in nonsolvent, and leading to phase separation that forms a solid polymer-rich membrane matrix and polymer-poor membrane pores. We demonstrate how mass-transfer-induced spinodal decomposition, thermal fluctuations, and glass-transition dynamics-implemented with mobility contrast between the polymer-rich and polymer-poor phases-are essential to the formation of asymmetric membrane microstructures. Specifically, we show that the competition between the propagation of the phase-separation and glass-transition fronts determines the degree of pore-size asymmetry. We also explore the sensitivity of these microstructures to the initial film composition, and compare their formation in 2D and 3D." @default.
• W3097349416 created "2020-11-09" @default.
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• W3097349416 date "2020-10-26" @default.
• W3097349416 modified "2023-10-16" @default.
• W3097349416 title "Mechanisms of Asymmetric Membrane Formation in Nonsolvent-Induced Phase Separation" @default.
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• W3097349416 doi "https://doi.org/10.1021/acsmacrolett.0c00609" @default.
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• W3097349416 hasPublicationYear "2020" @default.
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