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• W3097492039 startingPage "108285" @default.
• W3097492039 abstract "Two new polyoxometalates-based metal-organic complexes were synthesized, which display good adsorption activities toward organic dyes and bifunctional electrocatalysis activities. • The semi-rigid bis(pyrazine)-bis(amide) L is firstly introduced into the POMs. • Different POMs result in different architectures and properties of complexes 1 – 2 . • Complexes 1 – 2 possess good adsorption and desorption properties for organic dyes. • Complexes 1 – 2 exhibit good bifunctional electrocatalytic activities. Two new polyoxometalates (POMs)-based metal–organic complexes (MOCs), formula as [Cu 2 (L) 2 SiW 12 O 40 ] ( 1 ), [Cu(L)(β-Mo 8 O 26 ) 0.5 ]·H 2 O ( 2 ) [L = N,N′-bis(2-pyrazinecarboxamide)-1,2-cyclohexane] have been prepared by using a new semi-rigid bis(pyrazine)-bis(amide) ligand under the hydrothermal conditions. Crystal analysis reveals that complex 1 is a 2D supramolecular structure based on the 1D [CuL] n 2n+ chains, in which the [SiW 12 O 40 ] 4− (SiW 12 ) anions serve as noncoordinated templates. Complex 2 is a 2D network, which is composed of the bidentate bridging [β-Mo 8 O 26 ] 4− (Mo 8 ) anions and 1D [CuL] n 2n+ chains. Both 1 – 2 display excellent adsorption behaviors and can effectively adsorb organic dyes methylene blue (MB) and gentian violet (GV). It is worth mentioning that 1 – 2 were hardly changed after three cycles of the adsorption-desorption process. In addition, the bifunctional electrocatalytic performances of complex 1 – 2 were also studied in detail. The different architectures and properties of 1 – 2 were induced by diverse POM anions." @default.
• W3097492039 created "2020-11-09" @default.
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• W3097492039 date "2020-12-01" @default.
• W3097492039 modified "2023-10-16" @default.
• W3097492039 title "Two polyoxometalate-based CuII complexes with a new semi-rigid bis(pyrazine)-bis(amide) ligand: Architectures, adsorption activities for dyes and bifunctional electrocatalytic performances" @default.
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• W3097492039 doi "https://doi.org/10.1016/j.inoche.2020.108285" @default.
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