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• W3097531110 endingPage "19057" @default.
• W3097531110 startingPage "19052" @default.
• W3097531110 abstract "A single molecular rhodium catalyst system (PC2-Cp#RhIII) bearing two functional domains for both photosensitization and C–H carbometalation was designed to enable an intramolecular redox process. The hypothesized charge-transfer species (PC2•–-Cp#RhIV) was characterized by spectroscopic and electrochemical analyses. This photoinduced internal oxidation allows a facile access to the triplet state of the key post-transmetalation intermediate that readily undergoes C–C bond-forming reductive elimination with a lower activation barrier than in its singlet state, thus enabling catalytic C–H arylation and methylation processes." @default.
• W3097531110 created "2020-11-09" @default.
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• W3097531110 date "2020-10-30" @default.
• W3097531110 modified "2023-10-17" @default.
• W3097531110 title "Merging Two Functions in a Single Rh Catalyst System: Bimodular Conjugate for Light-Induced Oxidative Coupling" @default.
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• W3097531110 doi "https://doi.org/10.1021/jacs.0c09982" @default.
• W3097531110 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/33124802" @default.
• W3097531110 hasPublicationYear "2020" @default.
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