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• W3098096385 abstract "Clean hydrogen production through efficient and cost-effective electrochemical water splitting is highly promising to meeting future global energy demands. The design of Earth-abundant materials with both high activity for hydrogen evolution reaction (HER) and electrochemical stability in both acidic and alkaline environments summarize the outcomes needed for practical applications. Here, we report a non-noble 3d metal Cl-chemical doping of liquid phase exfoliated single/few-layer flakes of MoSe2 for creating MoSe2 nanoflakes/3d metal oxide-hydr(oxy)oxide hybrid HER-catalysts. We propose that the electron-transfer from MoSe2 nanoflakes to metal cations and the chlorine complexation-induced both neutralization, as well as the in situ formation of metal oxide-hydr(oxy)oxides on MoSe2 nanoflake's surface, tailor the proton affinity of the derived catalysts, increasing the number and HER-kinetic of their active sites in both acidic and alkaline electrolytes. The electrochemical coupling between the doped-MoSe2 nanoflakes/metal oxide-hydr(oxy)oxide hybrids and single-walled carbon nanotubes heterostructures further accelerates the HER process. Lastly, monolithic stacking of multiple heterostructures is reported as a facile electrode assembly strategy to achieve overpotential for a cathodic current density of 10mAcm-2 of 0.081V and 0.064V in 0.5M H2SO4 and 1M KOH, respectively. This opens up new opportunities to address the current density vs. overpotential requirements targeted in pH-universal H2 production." @default.
• W3098096385 created "2020-11-23" @default.
• W3098096385 creator A5004029612 @default.
• W3098096385 creator A5006596283 @default.
• W3098096385 creator A5009018237 @default.
• W3098096385 creator A5026332159 @default.
• W3098096385 creator A5050780974 @default.
• W3098096385 creator A5051997218 @default.
• W3098096385 creator A5063072946 @default.
• W3098096385 date "2018-08-08" @default.
• W3098096385 modified "2023-10-18" @default.
• W3098096385 title "Doped‐MoSe₂ Nanoflakes/3d Metal Oxide–Hydr(Oxy)Oxides Hybrid Catalysts for pH‐Universal Electrochemical Hydrogen Evolution Reaction" @default.
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