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• W3098539907 abstract "Significant molecular orientation can be achieved by time-symmetric single-cycle pulses of zero area, in the THz region. We show that in spite of the existence of a combined time-space symmetry operation, not only large peak instantaneous orientations but also nonzero time-average orientations over a rotational period can be obtained. We show that this unexpected phenomenon is due to interferences among eigenstates of the time-evolution operator, as was described previously for transport phenomena in quantum ratchets. This mechanism also works for sequences of identical pulses, spanning a rotational period. This fact can be used to obtain a net average molecular orientation regardless of the magnitude of the rotational constant." @default.
• W3098539907 created "2020-11-23" @default.
• W3098539907 creator A5008694962 @default.
• W3098539907 date "2012-07-24" @default.
• W3098539907 modified "2023-10-01" @default.
• W3098539907 title "Mechanism of molecular orientation by single-cycle pulses" @default.
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• W3098539907 doi "https://doi.org/10.1063/1.4736844" @default.
• W3098539907 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/22852614" @default.
• W3098539907 hasPublicationYear "2012" @default.
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