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• W3099014583 abstract "We study inelastic vibration-assisted charge transfer effects in two-site molecular junctions, focusing on signatures of vibrational anharmonicity on the electrical characteristics and the thermoelectric response of the junction. We consider three types of oscillators: harmonic, anharmonic-Morse allowing bond dissociation, and harmonic-quartic, mimicking a confinement potential. Using a quantum master equation method which is perturbative in the electron-vibration interaction, we find that the (inelastic) electrical and thermal conductances can be largely affected by the nature of the vibrational potential. In contrast, the Seebeck coefficient, the thermoelectric figure-of-merit, and the thermoelectric efficiency beyond linear response conceal this information, showing a rather weak sensitivity to vibrational anharmonicity. Our work illustrates that anharmonic (many-body) effects, consequential to the current-voltage characteristics, are of little effect for the thermoelectric performance in the present model." @default.
• W3099014583 created "2020-11-23" @default.
• W3099014583 creator A5007831957 @default.
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• W3099014583 date "2016-11-03" @default.
• W3099014583 modified "2023-09-23" @default.
• W3099014583 title "Effects of vibrational anharmonicity on molecular electronic conduction and thermoelectric efficiency" @default.
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• W3099014583 doi "https://doi.org/10.1063/1.4965824" @default.
• W3099014583 hasPublicationYear "2016" @default.
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