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• W3099101588 abstract "We present a new cavity-based polarimetric scheme for highly sensitive and time-resolved measurements of birefringence and dichroism, linear and circular, that employs rapidly-pulsed single-frequency CW laser sources and extends current cavity-based spectropolarimetric techniques. We demonstrate how the use of a CW laser source allows for gains in spectral resolution, signal intensity and data acquisition rate compared to traditional pulsed-based cavity ring-down polarimetry (CRDP). We discuss a particular CW-CRDP modality that is different from intensity-based cavity-enhanced polarimetric schemes as it relies on the determination of the polarization-rotation frequency during a ring-down event generated by large intracavity polarization anisotropies. We present the principles of CW-CRDP and validate the applicability of this technique for measurement of the non-resonant Faraday effect in solid SiO$_2$ and CeF$_3$ and gaseous butane. We give a general analysis of the fundamental sensitivity limits for CRDP techniques and show how the presented frequency-based methodology alleviates the requirement for high finesse cavities to achieve high polarimetric sensitivities, and, thus, allows for the extension of cavity-based polarimetric schemes into different spectral regimes but most importantly renders the CW-CRDP methodology particularly suitable for robust portable polarimetric instrumentations." @default.
• W3099101588 created "2020-11-23" @default.
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• W3099101588 date "2020-04-30" @default.
• W3099101588 modified "2023-10-11" @default.
• W3099101588 title "Continuous-wave cavity ring-down polarimetry" @default.
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• W3099101588 doi "https://doi.org/10.1063/5.0004476" @default.
• W3099101588 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/32357774" @default.
• W3099101588 hasPublicationYear "2020" @default.
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