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- W3100141828 abstract "The statistical mechanics of phase transitions in dense systems of polydisperse particles presents distinctive challenges to computer simulation and analytical theory alike. The core difficulty, namely dealing correctly with particle size fractionation between coexisting phases, is set out in the context of a critique of previous simulation work on such systems. Specialized Monte Carlo simulation techniques and moment free energy method calculations, capable of treating fractionation exactly, are then described and deployed to study the fluid-solid transition of an assembly of repulsive spherical particles described by a top-hat parent distribution of particle sizes. The cloud curve delineating the solid-fluid coexistence region is mapped as a function of the degree of polydispersity $delta$, and the properties of the incipient shadow phases are presented. The coexistence region is found to shift to higher densities as $delta$ increases, but does not exhibit the sharp narrowing predicted by many theories and some simulations." @default.
- W3100141828 created "2020-11-23" @default.
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- W3100141828 date "2010-12-09" @default.
- W3100141828 modified "2023-10-06" @default.
- W3100141828 title "Phase behavior of polydisperse spheres: Simulation strategies and an application to the freezing transition" @default.
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- W3100141828 doi "https://doi.org/10.1063/1.3510534" @default.
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