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- W3100202236 abstract "We investigate local phase transitions of the solvent in the neighborhood of a solvophobic polymer chain which is induced by a change of the polymer-solvent repulsion and the solvent pressure in the bulk solution. We describe the polymer in solution by the Edwards model, where the conditional partition function of the polymer chain at a fixed radius of gyration is described by a mean-field theory. The contributions of the polymer-solvent and the solvent-solvent interactions to the total free energy are described within the mean-field approximation. We obtain the total free energy of the solution as a function of the radius of gyration and the average solvent number density within the gyration volume. The resulting system of coupled equations is solved varying the polymer-solvent repulsion strength at high solvent pressure in the bulk. We show that the coil-globule (globule-coil) transition occurs accompanied by a local solvent evaporation (condensation) within the gyration volume" @default.
- W3100202236 created "2020-11-23" @default.
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- W3100202236 date "2014-11-26" @default.
- W3100202236 modified "2023-10-18" @default.
- W3100202236 title "The local phase transitions of the solvent in the neighborhood of a solvophobic polymer at high pressures" @default.
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- W3100202236 doi "https://doi.org/10.1063/1.4902092" @default.
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