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• W3100236365 abstract "Hydrogen is rarely observed as ligand in hypervalent species, however, we find that high-pressure hydrogenation may stabilise hypervalent hydrogen-rich materials. Focussing on ternary silicon hydrides via lithium doping, we find anions composed of hypervalent silicon with H ligands formed under high pressure. Our results reveal two new hypervalent anions: layered-SiH$_{5}^{-}$ and tricapped trigonal prismatic SiH$_{6}^{2-}$. These differ from octahedral SiH$_{6}^{2-}$ described in earlier studies. In addition, there are further hydrogen-rich structures Li$_{3}$SiH$_{10}$ and Li$_{2}$SiH$_{6+delta}$ which may be stabilised at high pressure. Our work provides pointers to future investigations on hydrogen-rich materials." @default.
• W3100236365 created "2020-11-23" @default.
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• W3100236365 date "2020-11-18" @default.
• W3100236365 modified "2023-10-09" @default.
• W3100236365 title "Ternary hypervalent silicon hydrides via lithium at high pressure" @default.
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• W3100236365 doi "https://doi.org/10.1103/physrevmaterials.4.113607" @default.
• W3100236365 hasPublicationYear "2020" @default.
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