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• W3100340839 abstract "The fundamental O-D stretch region (2600 - 2800 cm-1) of the fully deuterated water dimer, (D2O)2, is studied using a pulsed supersonic slit jet source and a tunable optical parametric oscillator source. Relatively high spectral resolution (0.002 cm-1) enables all six dimer tunneling components to be observed, in most cases, for the acceptor asymmetric O-D stretch, the donor free O-D stretch, and the donor bound O-D stretch vibrations. The dominant acceptor switching tunneling splittings are observed to decrease moderately in the excited O-D stretch states, to roughly 75% of their ground state values, whereas the smaller donor-acceptor interchange splittings show more dramatic and irregular decreases. Excited state predissociation lifetimes, as determined from observed line broadening, show large variations (0.2 to 5 nanoseconds) depending on vibrational state, K-value, and tunneling symmetry. Another very weak band is tentatively assigned to a combination mode involving an intramolecular O-D stretch plus an intermolecular twist overtone. Asymmetric O-D stretch bands of the mixed isotopologue dimers D2O-DOH and D2O-HOD are also observed and analyzed." @default.
• W3100340839 created "2020-11-23" @default.
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• W3100340839 date "2019-04-26" @default.
• W3100340839 modified "2023-09-30" @default.
• W3100340839 title "Spectra of the D2O dimer in the O–D fundamental stretch region: Vibrational dependence of tunneling splittings and lifetimes" @default.
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• W3100340839 doi "https://doi.org/10.1063/1.5092503" @default.
• W3100340839 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31042915" @default.
• W3100340839 hasPublicationYear "2019" @default.
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