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- W3100349601 abstract "The transition metal dichalcogenide TiSe$_2$ has received significant research attention over the past four decades. Different studies have presented ways to suppress the 200~K charge density wave transition, vary low temperature resistivity by several orders of magnitude, and stabilize magnetism or superconductivity. Here we give the results of a new synthesis technique whereby samples were grown in a high pressure environment with up to 180~bar of argon gas. Above 100~K, properties are nearly unchanged from previous reports, but a hysteretic resistance region that begins around 80~K, accompanied by insulating low temperature behavior, is distinct from anything previously observed. An accompanying decrease in carrier concentration is seen in Hall effect measurements, and photoemission data show a removal of an electron pocket from the Fermi surface in an insulating sample. We conclude that high inert gas pressure synthesis accesses an underlying nonmetallic ground state in a material long speculated to be an excitonic insulator." @default.
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- W3100349601 date "2019-05-14" @default.
- W3100349601 modified "2023-10-18" @default.
- W3100349601 title "Intrinsic insulating ground state in transition metal dichalcogenide <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msub><mml:mrow><mml:mi>TiSe</mml:mi></mml:mrow><mml:mn>2</mml:mn></mml:msub></mml:math>" @default.
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- W3100349601 doi "https://doi.org/10.1103/physrevmaterials.3.053402" @default.
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