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• W3100406469 abstract "We study discrete solvent effects on the interaction of two parallel charged surfaces in ionic aqueous solution. These effects are taken into account by adding a bilinear non-local term to the free energy of Poisson-Boltzmann theory. We study numerically the density profile of ions between the two plates, and the resulting inter-plate pressure. At large plate separations the two plates are decoupled and the ion distribution can be characterized by an effective Poisson-Boltzmann charge that is smaller than the nominal charge. The pressure is thus reduced relative to Poisson-Boltzmann predictions. At plate separations below ~2 nm the pressure is modified considerably, due to the solvent mediated short-range attraction between ions in the the system. For high surface charges this contribution can overcome the mean-field repulsion giving rise to a net attraction between the plates." @default.
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• W3100406469 date "2001-02-15" @default.
• W3100406469 modified "2023-09-23" @default.
• W3100406469 title "Discrete aqueous solvent effects and possible attractive forces" @default.
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• W3100406469 doi "https://doi.org/10.1063/1.1331569" @default.
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