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• W3100498474 abstract "Abstract In order to establish the universality of the excess heat production in electrochemical reaction, under a high magnetic field, as one of the most fundamental electrochemical reactions, the case of ferricyanide-ferrocyanide redox reaction was examined, where ionic vacancies with ± 1 unit charge were collided by means of magnetohydrodynamic (MHD) flow. As a result, from the pair annihilation of the vacancies with opposite signs, beyond 7 T, excess heat production up to 25 kJ·mol −1 in average at 15 T was observed, which was attributed to the liberation of the solvation energy stored in a pair of the vacancy cores with a 0.32 nm radius, i.e., 112 kJ·mol −1 . Difference between the observed and expected energies comes from the small collision efficiency of 0.22 due to small radius of the vacancy core. Ionic vacancy initially created as a by-product of electrode reaction is unstable in solution phase, stabilized by releasing solvation energy. Ionic vacancy utilizes the energy to enlarge the core and stores the energy in it. As a result, solvated ionic vacancy consists of a polarized free space of the enlarged core surrounded by oppositely charged ionic cloud. The accuracy and precision of the measured values were ascertained by in situ standard additive method." @default.
• W3100498474 created "2020-11-23" @default.
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• W3100498474 date "2020-11-18" @default.
• W3100498474 modified "2023-09-25" @default.
• W3100498474 title "Excess heat production in the redox couple reaction of ferricyanide and ferrocyanide" @default.
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• W3100498474 doi "https://doi.org/10.1038/s41598-020-76611-3" @default.
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