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• W3100505554 abstract "Abstract The strong coupling between intense laser fields and valence electrons in molecules causes distortions of the potential energy hypersurfaces which determine the motion of the nuclei and influence possible reaction pathways. The coupling strength varies with the angle between the light electric field and valence orbital, and thereby adds another dimension to the effective molecular potential energy surface, leading to the emergence of light-induced conical intersections. Here, we demonstrate that multiphoton couplings can give rise to complex light-induced potential energy surfaces that govern molecular behavior. In the laser-induced dissociation of H 2 + , the simplest of molecules, we measure a strongly modulated angular distribution of protons which has escaped prior observation. Using two-color Floquet theory, we show that the modulations result from ultrafast dynamics on light-induced molecular potentials. These potentials are shaped by the amplitude, duration and phase of the dressing fields, allowing for manipulating the dissociation dynamics of small molecules." @default.
• W3100505554 created "2020-11-23" @default.
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• W3100505554 date "2020-05-22" @default.
• W3100505554 modified "2023-10-18" @default.
• W3100505554 title "Probing multiphoton light-induced molecular potentials" @default.
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• W3100505554 doi "https://doi.org/10.1038/s41467-020-16422-2" @default.
• W3100505554 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/7244592" @default.
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