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- W3100602804 abstract "Coherent coupling between spatially separated systems has long been explored as a necessary requirement for quantum information and cryptography. Recent discoveries suggest such phenomena appear in a much wider range of processes, including light-harvesting in photosynthesis. These discoveries have been facilitated by developments in coherent multi-dimensional spectroscopy (CMDS) that allow interactions between different electronic states to be identified in crowded spectra. For complex systems, however, spectral broadening and multiple overlapping peaks limit the ability to separate, identify and properly analyse all contributions. Here we demonstrate how pathway-selective CMDS can overcome these limitations to reveal, isolate and allow detailed analysis of weak coherent coupling between spatially separated excitons localised to different semiconductor quantum wells. Selective excitation of the coherence pathways, by spectrally shaping the laser pulses, provides access to previously hidden details and enables quantitative analysis that can facilitate precise and detailed understanding of interactions in this and other complex systems." @default.
- W3100602804 created "2020-11-23" @default.
- W3100602804 creator A5053942567 @default.
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- W3100602804 date "2014-03-14" @default.
- W3100602804 modified "2023-09-30" @default.
- W3100602804 title "Isolating quantum coherence using coherent multi-dimensional spectroscopy with spectrally shaped pulses" @default.
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- W3100602804 doi "https://doi.org/10.1364/oe.22.006719" @default.
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