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• W3100606416 abstract "The proper design of DNA sequences allows for the formation of well-defined supramolecular units with controlled interactions via a consecution of self-assembling processes. Here, we benefit from the controlled DNA self-assembly to experimentally realize particles with well-defined valence, namely, tetravalent nanostars (A) and bivalent chains (B). We specifically focus on the case in which A particles can only bind to B particles, via appropriately designed sticky-end sequences. Hence AA and BB bonds are not allowed. Such a binary mixture system reproduces with DNA-based particles the physics of poly-functional condensation, with an exquisite control over the bonding process, tuned by the ratio, r, between B and A units and by the temperature, T. We report dynamic light scattering experiments in a window of Ts ranging from 10 °C to 55 °C and an interval of r around the percolation transition to quantify the decay of the density correlation for the different cases. At low T, when all possible bonds are formed, the system behaves as a fully bonded network, as a percolating gel, and as a cluster fluid depending on the selected r." @default.
• W3100606416 created "2020-11-23" @default.
• W3100606416 creator A5016143876 @default.
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• W3100606416 date "2018-01-09" @default.
• W3100606416 modified "2023-10-17" @default.
• W3100606416 title "Binding branched and linear DNA structures: From isolated clusters to fully bonded gels" @default.
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• W3100606416 doi "https://doi.org/10.1063/1.5011720" @default.
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• W3100606416 hasPublicationYear "2018" @default.
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