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- W3100648491 abstract "We predict the enhanced light harvesting of a protein-pigment complex when assembled to a quantum dot (QD) antenna. Our prototypical nanoassembly setup is composed of a Fenna-Mattews-Olson system hosting 8 Bacteriochlorophyll (BChl) a dyes, and a near-infrared emitting CdSe <inf xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>x</inf> Te <inf xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>(1−x)</inf> /ZnS alloy-core/shell nanocrystal. BChl a has two wide windows of poor absorption in the green and orange-red bands, precisely where most of the sunlight energy lies. The selected QD is able to collect sunlight efficiently in a broader band and funnel its energy by a (non-radiative) Förster resonance energy transfer mechanism to the dyes embedded in the protein. By virtue of the coupling between the QD and the dyes, the nanoassembly absorption is dramatically improved in the poor absorption window of the BChl a." @default.
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- W3100648491 date "2018-11-01" @default.
- W3100648491 modified "2023-09-23" @default.
- W3100648491 title "Enhanced light-harvesting of protein-pigment complexes assisted by a quantum dot antenna*" @default.
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- W3100648491 doi "https://doi.org/10.1109/nanofim.2018.8688607" @default.
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