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- W3100723909 abstract "It has been widely acknowledged that the Li4SiO4-based adsorbents with smaller particle size and tailored structure will certainly exhibit superior CO2 capture performance. In this work, a novel two-phase synthesis method was proposed to produce tailored micro-scale Li4SiO4-based adsorbents with ultrafast CO2 capture rate. The effects of synthetic temperature on the phase compositions, the chemical bonds, the pore structure, the surface morphology and the CO2 capture performance of obtained adsorbents were systematically investigated. It is found that the increase of temperature during synthesis process could promote the Li4SiO4 content of obtained adsorbents. Nevertheless, higher temperature also leads to the aggravation and sintering of particles, thus hindering the capacity of adsorbents. Examining the pros and cons, the adsorbent calcined at 600 °C shows the greatest morphology consisted of hollow-structured microspheres with a uniform diameter of 1–2 μm and exhibits the fastest adsorption rate as well as the highest adsorption capacity (~ 0.184 g CO2/g adsorbent within only 5 min's adsorption under 15 vol% CO2), leading to a superior Li4SiO4 conversion as high as ~80%. In a word, this two-phase method is promising in the future production of Li4SiO4-based microspheres for high-efficient and ultrafast CO2 capture." @default.
- W3100723909 created "2020-11-23" @default.
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- W3100723909 date "2021-03-01" @default.
- W3100723909 modified "2023-09-26" @default.
- W3100723909 title "Novel synthesis of tailored Li4SiO4-based microspheres for ultrafast CO2 adsorption" @default.
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- W3100723909 doi "https://doi.org/10.1016/j.fuproc.2020.106675" @default.
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