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• W3101218921 abstract "We present a 100 kHz broadband vibrational sum-frequency generation (VSFG) spectrometer operating in the 5.5-10.5 $mu$m (950-1750 cm$^{-1}$) wavelength range. The mid-infrared beam of the system is obtained from a collinear, type-I LiGaS$_{2}$ crystal based optical parametric amplifier seeded by a supercontinuum and pumped directly by 180 fs, ~32 $mu$J, 1.03 $mu$m pulses from an Yb:KGd(WO$_{4}$)$_{2}$ laser system. Up to 0.5 $mu$J mid-infrared pulses with durations below 100 fs were obtained after dispersion compensation utilizing bulk materials. We demonstrate the utility of the spectrometer by recording high-resolution, low-noise vibrational spectra of Langmuir-Blodgett supported lipid monolayers on CaF$_{2}$. The presented VSFG spectrometer scheme offers superior signal-to-noise ratios and constitutes a high-efficiency, low-cost, easy-to-use alternative to traditional schemes relying on optical parametric amplification followed by difference frequency generation." @default.
• W3101218921 created "2020-11-23" @default.
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• W3101218921 date "2019-05-13" @default.
• W3101218921 modified "2023-10-16" @default.
• W3101218921 title "Broadband vibrational sum-frequency generation spectrometer at 100 kHz in the 950-1750 cm⁻¹ spectral range utilizing a LiGaS₂ optical parametric amplifier" @default.
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• W3101218921 doi "https://doi.org/10.1364/oe.27.015289" @default.
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