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• W3101223670 abstract "In this paper we show that the virial expansion up to third order for the osmotic pressure of a dilute polymer solution, including first-order perturbative corrections to the virial coefficients, allows for a scaling description of phase-separation data for polymer solutions in reduced variables. This scaling description provides a method to estimate the Θ-temperature, where demixing occurs in the limit of vanishing polymer volume fraction φ and infinite chain length N, without explicit assumptions concerning the chain-length dependence of the critical parameters Tc and φc. The scaling incorporates three limiting regimes: The Ising limit asymptotically close to the critical point of phase separation, the pure-solvent limit, and the tricritical limit for the polymer-rich phase asymptotically close to the theta point. We incorporate the effects of critical and tricritical fluctuations on the coexistence-curve scaling by using renormalization-group methods. We present a detailed comparison with experimental and simulation data for coexistence curves and compare our estimates for the Θ-temperatures of several systems with those obtained from different extrapolation schemes." @default.
• W3101223670 created "2020-11-23" @default.
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• W3101223670 date "2002-09-04" @default.
• W3101223670 modified "2023-09-24" @default.
• W3101223670 title "Scaling of demixing curves and crossover from critical to tricritical behavior in polymer solutions" @default.
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• W3101223670 doi "https://doi.org/10.1063/1.1502249" @default.
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