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• W3101523364 abstract "We apply a new formalism to derive the higher-order quantum kinetic expansion (QKE) for studying dissipative dynamics in a general quantum network coupled with an arbitrary thermal bath. The dynamics of system population is described by a time-convoluted kinetic equation, where the time-nonlocal rate kernel is systematically expanded of the order of off-diagonal elements of the system Hamiltonian. In the second order, the rate kernel recovers the expression of the noninteracting-blip approximation method. The higher-order corrections in the rate kernel account for the effects of the multi-site quantum coherence and the bath relaxation. In a quantum harmonic bath, the rate kernels of different orders are analytically derived. As demonstrated by four examples, the higher-order QKE can reliably predict quantum dissipative dynamics, comparing well with the hierarchic equation approach. More importantly, the higher-order rate kernels can distinguish and quantify distinct nontrivial quantum coherent effects, such as long-range energy transfer from quantum tunneling and quantum interference arising from the phase accumulation of interactions." @default.
• W3101523364 created "2020-11-23" @default.
• W3101523364 creator A5032708958 @default.
• W3101523364 creator A5049476042 @default.
• W3101523364 date "2013-07-23" @default.
• W3101523364 modified "2023-09-30" @default.
• W3101523364 title "Higher-order kinetic expansion of quantum dissipative dynamics: Mapping quantum networks to kinetic networks" @default.
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• W3101523364 doi "https://doi.org/10.1063/1.4812781" @default.
• W3101523364 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/23901955" @default.
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