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- W3102145108 abstract "A recent polarized neutron diffraction experiment on the $5{d}^{2}$ rhenium double perovskite ${mathrm{Ba}}_{2}mathrm{YRe}{mathrm{O}}_{6}$ held at a low temperature uncovered weak magnetic diffraction peaks. Data analysis inferred a significantly reduced Re dipole moment, and long-range order compatible with an antiferromagnetic, noncollinear motif. To interpret the experimental findings, we present a model wave function for Re ions derived from the crystal field potential, Coulomb interaction, and spin-orbit coupling that fully respects the symmetry of the low-temperature ordered state. It is used to calculate in analytic form all multipole moments visible in neutron and resonance enhanced x-ray diffraction. A minimal model consistent with available neutron diffraction data predicts significant multipolar moments up to the hexadecapole and, in particular, a dominant chargelike quadrupole moment. Calculated diffraction patterns embrace single crystal x-ray diffraction at the Re $L$ edge, and renewed neutron diffraction, to probe the presumed underlying multipolar order." @default.
- W3102145108 created "2020-11-23" @default.
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- W3102145108 date "2021-03-19" @default.
- W3102145108 modified "2023-09-27" @default.
- W3102145108 title "Diffraction by multipoles in a <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:mrow><mml:mn>5</mml:mn><mml:msup><mml:mi>d</mml:mi><mml:mn>2</mml:mn></mml:msup></mml:mrow></mml:math> rhenium double perovskite" @default.
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- W3102145108 doi "https://doi.org/10.1103/physrevb.103.104429" @default.
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