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• W3102174372 abstract "The interpretation of nanoplasmonic effects on molecular properties, such as metal-enhanced absorption or fluorescence, typically assumes a fully coherent picture (in the quantum-mechanical sense) of the phenomena. Yet, there may be conditions where the coherent picture breaks down, and the decoherence effect should be accounted for. Using a state-of-the-art multiscale model approach able to include environment-induced dephasing, here we show that metal nanoparticle effects on the light absorption by a nearby molecule is strongly affected (even qualitatively, i.e., suppression vs enhancement) by molecular electronic decoherence. The present work shows that decoherence can be thought of as a further design element of molecular nanoplasmonic systems." @default.
• W3102174372 created "2020-11-23" @default.
• W3102174372 creator A5037684430 @default.
• W3102174372 creator A5078141074 @default.
• W3102174372 date "2019-07-26" @default.
• W3102174372 modified "2023-09-26" @default.
• W3102174372 title "Role of coherence in the plasmonic control of molecular absorption" @default.
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• W3102174372 doi "https://doi.org/10.1063/1.5109378" @default.
• W3102174372 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31370514" @default.
• W3102174372 hasPublicationYear "2019" @default.
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