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• W3102344327 endingPage "405601" @default.
• W3102344327 startingPage "405601" @default.
• W3102344327 abstract "We report the bulk magnetic properties of a yet unexplored vanadium-based multivalued spinel system, Zn3V3O8. A Curie-Weiss fit of our dc magnetic susceptibility data in the temperature region from 140 to 300 K yields a Curie constant C = 0.75cm3K/mole V, theta CW = -370 K. We have observed a splitting between the zero field cooled ZFC and field cooled FC susceptibility curves below a temperature Tirr of about 6.3 K. The value of the 'frustration parameter' nearly equals to 100 suggests that the system is strongly frustrated. From the ac susceptibility measurements we find a logarithmic variation of freezing temperature (Tf ) with frequency attesting to the formation of a spin glass below Tf . However, the value of the characteristic frequency obtained from the Vogel-Fulcher fit suggests that the ground state is closer to a cluster glass rather than a conventional spin glass. We explored further consequences of the spin glass behavior and observed aging phenomena and memory effect (both in ZFC and FC). We found that a positive temperature cycle erases the memory, as predicted by the hierarchical model. From the heat capacity CP data, a hump-like anomaly was observed in CP /T at about 3.75 K. Below this temperature the magnetic heat capacity shows a nearly linear dependence with T which is consistent with the formation of a spin glass state below Tf in Zn3V3O8." @default.
• W3102344327 created "2020-11-23" @default.
• W3102344327 creator A5003537920 @default.
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• W3102344327 date "2014-09-11" @default.
• W3102344327 modified "2023-09-30" @default.
• W3102344327 title "Cluster spin glass behavior in geometrically frustrated Zn₃V₃O₈" @default.
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• W3102344327 doi "https://doi.org/10.1088/0953-8984/26/40/405601" @default.
• W3102344327 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/25210922" @default.
• W3102344327 hasPublicationYear "2014" @default.
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