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• W3102501864 abstract "Recently, the dry reforming of methane (DRM) has received much attention as a conversion technology of greenhouse gases. Ni-based catalysts supported on ternary metal oxide composite (ZrTiAlOx) were prepared to improve the coke resistance properties in the DRM (CH4:CO2 = 1) at low temperature. The ZrTiAlOx supports with different ratios of Zr/Ti were prepared through the modified Pechini sol-gel method, and then the Ni was impregnated on the synthesized support via the incipient wetness impregnation method. Considering the Zr/Ti ratios, different catalytic activity and durability in the DRM were identified. The Ni/ZrTiAlOx catalyst with Zr/Ti of 2 exhibited enhanced coke inhibition property compared to the others at low temperature DRM for 50 h. The catalysts with a high Zr/Ti ratio under the same condition were rapidly deactivated, while the catalyst with a low Zr/Ti ratio showed deficient activity. It was found from temperature-programmed surface reactions (TPSR) and DRIFTS (Diffuse Reflectance Infrared Fourier Transform Spectroscopy) analysis that the addition of Ti has led in to higher catalytic stability at Zr/Ti = 2, which could be as a result of oxygen vacancies generated by the ternary metal oxides. Ni/ZrTiAlOx catalyst with ratio of Zr/Ti = 2 showed high stability and good catalytic activity towards DRM for the production of syngas." @default.
• W3102501864 created "2020-11-23" @default.
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• W3102501864 date "2020-11-17" @default.
• W3102501864 modified "2023-09-27" @default.
• W3102501864 title "Preparation and Characterization of Ni/ZrTiAlOx Catalyst via Sol-Gel and Impregnation Methods for Low Temperature Dry Reforming of Methane" @default.
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• W3102501864 doi "https://doi.org/10.3390/catal10111335" @default.
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